Phonon Driven Nonlinear Electrical Behavior in Molecular Devices

Data di pubblicazione: 28 Set 2007

RivistaFonte dati: OPENALEXTipo OpenAlex: articleOpen Access

Electronic transport in a model molecular device coupled to local phonon modes is theoretically analyzed. The method allows for obtaining an accurate approximation of the system’s quantum state irrespective of the electron and phonon energy scales. Nonlinear electrical features emerge from the calculated current-voltage characteristics. The quantum corrections with respect to the adiabatic limit characterize the transport scenario, and the polaronic reduction of the effective device-lead coupling plays a fundamental role in the unusual electrical features.

Editore
American Physical Society
Fonte
Physical review letters
Volume
99
Fascicolo
13
Pagine
136404
Citazioni
32
ID archivio
953999186c8a06622c924e6872738061
Riferimenti
Volume: 99 Issue: 13 Pages: 136404